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1 article(s) from Elmas, Sait

Anion effect controlling the selectivity in the zinc-catalysed copolymerisation of CO₂ and cyclohexene oxide

Sait Elmas,
Muhammad Afzal Subhani,
Walter Leitner and
Thomas E. Müller

Beilstein J. Org. Chem. 2015, 11, 42–49, doi:10.3762/bjoc.11.7

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Graphical Abstract

Scheme 1: Structural motif of two important types of catalysts and typical substrate specificity in the copol...

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Scheme 2: Binuclear Zn(II) complexes [LZn₂](CF₃SO₃)₂ (1, KOP113) and [LZn₂](p-TSO₃)₂ (2, KOP115) explored in ...

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Scheme 3: Copolymerisation of CO₂ and cyclohexene oxide (*: end groups of the polymer chain).

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Figure 1: Time-resolved IR spectra of the copolymerisation of CO₂ and CHO with catalyst 1 showing the formati...

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Figure 2: Time–concentration profile of the copolymerisation of CO₂ and CHO in the presence of catalytic amou...

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Figure 3: Carbonate region of the time-resolved IR spectra recorded during the copolymerisation of CO₂ and cy...

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Figure 4: Time–concentration profile of the copolymerisation of CO₂ and CHO in the presence of catalytic amou...

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Scheme 4: Proposed inner-sphere mechanism for the copolymerisation of CO₂ and CHO with binuclear zinc complex...

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Published 12 Jan 2015

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Anion effect controlling the selectivity in the zinc-catalysed copolymerisation of CO2 and cyclohexene oxide

Anion effect controlling the selectivity in the zinc-catalysed copolymerisation of CO₂ and cyclohexene oxide